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Theoretical and experimental investigation of the electron affinities of allene and propyne

โœ Scribed by B. Ciommer; K.M. Nguyen; H. Schwarz; G. Frenking; G. Kwiatkowski; E. Illenberger

Publisher
Elsevier Science
Year
1985
Tongue
English
Weight
45 KB
Volume
114
Category
Article
ISSN
0009-2614

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Theoretical and experimental investigati
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In qualitative agreement with semi-empirical (MNDO) and ab initio calculations, the electron affinities measured by electron transmission spectroscopy are found to be strongly negative for allene (-1.9 -+ 0.1 eV) and propyne (-2.8 -+ 0.1 eV)

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The ignition delays of insaturated hydrocarbons-oxygen-argon mixtures were measured behind shock waves in the cases of acetylene, propyne, allene and 1,3-butadiene. Reflected shock waves permitted to obtain temperatures from 1000-1650 K and pressures from 8.5 to 10.0 atm. A particular effort has be