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The Townes and Dailey approach to the interpretation of NQR parameters in the light of non-empirical calculations. Three-membered rings

✍ Scribed by M. Yu. Balakina; O. D. Fominykh; I. D. Morozova; D. Ya. Osokin


Publisher
John Wiley and Sons
Year
1995
Tongue
English
Weight
485 KB
Volume
33
Category
Article
ISSN
0749-1581

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✦ Synopsis


Abstract

The nuclear and electronic contributions to the EFG tensor components eq~ii~ at ^14^N, ^17^O, ^33^S and ^35^Cl nuclei in aziridine, methylaziridine, chloroaziridine, oxirane and thiirane were determined. The nuclear contributions were calculated within classical representations, while electronic contributions were calculated non‐empirically using a 6–31G* basis set within the framework of the LMO approach. On the basis of the analysis of the contributions to the EFG tensor components from definite bond and lone‐pair orbitals, the main concepts of the Townes and Dailey approach were tested.