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The theoretical description of an asymmetric, nonresonant charge transfer process; Li + Na+ ⇌ Li+ + Na the two-state approximation

✍ Scribed by Carl F. Melius; William A. Goddard III


Publisher
Elsevier Science
Year
1972
Tongue
English
Weight
401 KB
Volume
15
Category
Article
ISSN
0009-2614

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✦ Synopsis


The charge transfer process for the collision Li + Na ÷ ~ Li ÷ + Na has been studied theoretically by a two-state, impact parameter approach using molecular wavefunctions. Including the coupling term (4 lla/aRI¢,2> due to the breakdown of the Born-Oppenheimer approximation,we obtain total charge transfer cross sections in good agreement with experimental results.