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The Synthesis of Pseudo-Geminal, Pseudo-Ortho and Ortho Hydroxy-oxazolinyl[2.2]paracyclophanes for Use as Ligands in Asymmetric Catalysis

✍ Scribed by Carsten Bolm; Daniel K. Whelligan


Publisher
John Wiley and Sons
Year
2006
Tongue
English
Weight
145 KB
Volume
348
Category
Article
ISSN
1615-4150

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✦ Synopsis


Abstract

Synthetic routes to pseudo‐geminal, pseudo‐ortho and ortho hydroxy‐oxazolinyl[2.2]paracyclophanes (and the diastereoisomers of each) for use as N,O ligands in asymmetric catalysis have been devised. The substitution pattern was found to have a strong effect on the rate and enantioselectivity of the formed catalyst in the addition of diethylzinc to benzaldehyde.