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The synthesis of a benzamidine-containing NR2B-selective NMDA receptor ligand labelled with tritium or fluorine-18

✍ Scribed by Terence G. Hamill; John A. McCauley; H. Donald Burns


Publisher
John Wiley and Sons
Year
2005
Tongue
French
Weight
118 KB
Volume
48
Category
Article
ISSN
0022-2135

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✦ Synopsis


Abstract

A novel tritium or flourine‐18‐labelled benzamidine‐containing NR2B‐selective NMDA receptor ligand has been synthesized. This compound was designed to contain the fluoromethoxy group to allow for the synthesis of a high specific activity, fluorine‐18‐labelled PET tracer for imaging studies of the NR2B receptor. In addition to the fluorine‐18‐labelled compound, this compound was also tritium labelled. The tritiated ligand (11 Ci/mmol) was synthesized by a gas tritiation reaction of an aryl bromide precursor. The fluorine‐18 ligand (2916 Ci/mmol), which was deuterated in the fluoromethoxy group to aid in metabolic stability, was synthesized by alkylating a phenolic precursor with [^18^F]fluoromethylbromide‐d~2~. Copyright © 2004 John Wiley & Sons, Ltd.