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The surface modification of polyethylene by solution-phase photochemical grafting using short irradiation times

✍ Scribed by L. M. Hamilton; A. Green; S. Edge; J. P. S. Badyal; W. J. Feast; W. F. Pacynko


Publisher
John Wiley and Sons
Year
1994
Tongue
English
Weight
520 KB
Volume
52
Category
Article
ISSN
0021-8995

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✦ Synopsis


The surface modification of low-density polyethylene by solution-phase photochemical grafting with acrylic acid and acrylamide is described. After irradiation for 3 min, the contact angles of the modified surfaces with water were ca. 20, 30, and 40°C and ca. 40, 40, and 80°C for grafting solutions containing 2 M , 1 M , and 0.1M of acrylamide and acrylic acid respectively. X-Ray photoelectron spectroscopy (XPS) and attenuated total reflectance infrared spectroscopy ( ATRIR) of the modified polyethylene surfaces were consistent with the presence of grafts of polyacrylamide or poly (acrylic acid). Grafting using low concentrations of monomers, that is, O.lM, resulted in a small, 20' decrease in contact angle for grafting with acrylic acid but a larger, 60" decrease for acrylamide. 0 1994