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The stability of hydrogen atoms in irradiated aqueous solutions

✍ Scribed by C.J. Ultee; C.R. Kepford

Publisher
Elsevier Science
Year
1969
Tongue
English
Weight
184 KB
Volume
3
Category
Article
ISSN
0009-2614

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✦ Synopsis

The decay oi H-atoms in several y-irradiated aqueous solutions was examined by ESR spectroscopy from 'UΒ°K to 150Β°K. In perchloric acid the decay indicates the presence of two trapping sites. The more strongly trapped H-atoms decay by a first-order process, apparently resulting from a slow release from the traps followed by a fast reaction.

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Isotope effects in the yields of H-and D-atoms in acid, neutral and alkaline matrices lwe been studied bp EPR merhods. In acid matrices the isotope effect is the same in UV-and X-irmdiated matrices, but in neutral and alhaline m&rices the effect is Iarger in UV-irradiated matrices. Furthermore, \\he