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The polyketide folding mode in the biogenesis of isoshinanolone and plumbagin from Ancistrocladus heyneanus (Ancistrocladaceae)

✍ Scribed by Gerhard Bringmann; Michael Wohlfarth; Heiko Rischer; Markus Rückert; Jan Schlauer


Book ID
104260150
Publisher
Elsevier Science
Year
1998
Tongue
French
Weight
234 KB
Volume
39
Category
Article
ISSN
0040-4039

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✦ Synopsis


The biosynthetic origins of the tetralone isoshinanolone and the related naphthoquinone phimbagin were investigated by feeding [13C2]-acetate to suspended callus cultures of Ancistrocladus heyneanus. The orientation of the acetate subunits was elucidated by a similax experiment using [2-~3C]-acetate. The polyketide folding mode found for isoshinanolonc and plumbagin constitutes a further hint at the acetogenic nature of the naphthylisoquinoline alkaloids, which are typical of A.

heyneanus and other species of Ancistrocladaceac and Dioacophyllaceae.