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The Photochemical Behavior of Endocyclic Oxa-enones with Substituents on the CC Double Bond. (Preliminary communication)

✍ Scribed by Paul Margaretha


Publisher
John Wiley and Sons
Year
1974
Tongue
German
Weight
361 KB
Volume
57
Category
Article
ISSN
0018-019X

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✦ Synopsis


Abstract

Alkyl substituents on C~β~ of the CC double bond hinder both photodimerization of endocyclic oxa‐enones (14) and their photocycloaddition to olefins, and they cause a loss of regiospecificity in dimerization in unpolar solvents. The oxa‐enone 3 which like the bicyclic compounds 4 fails to dimerize at all, is shown to incorporate deuterium at the tertiary isopropyl carbon atom in CD~3~OD solution as a consequence of a bimolecularly initiated photoenolization.