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The mechanism of warfarin formation from 4-hydroxycoumarin and β-anilinobenzylacetone. Evidence for schiff base intermediates showing enhanced reactivity in the Michael reaction

✍ Scribed by Collin Schroeder; Seymour Preis; Karl Paul Link


Publisher
Elsevier Science
Year
1960
Tongue
French
Weight
338 KB
Volume
1
Category
Article
ISSN
0040-4039

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✦ Synopsis


PREVlOUS kinetic studies' have shown that the formation of warfarin (I) from 4-hydroxycoumarin (II) and S-anilinobenzglacetone (III) in the presence of aniline (reaction 1) is more rapid (ca. double at equivalent concentrations) ? 'cs"a C6 H,-fkl-CH&-CH3 CgHg -NH2 C6H5-NH x 'III I than its formation from 4-hydroxycoumarin and benzalacetone (IV) in the presence of aniline (reaction 2). 1 In the Japanese Patent Court demandant Toko Chemical Co., Ltd., Tokyo, Japan, for H. Naruke "on the scope of right of patent number 195, Ok0 held by Wisconsin Alumni Research Foundation, Madison 5, Wisconsin, Trial No. 3800/1953" dated October 26, 1953, it is asserted that the formation of narfarin from 4-hydroqxoumarin and B-anilinobenzylacetone is a direct (S > reaction. 2 2 The chemical name 3-(cc-acetonylbenzyl)-4-hydroxycoumari.n is the systematic name selected by Chemical Abstracts for the anticoagulant warfarin.