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The Interplay of Hydrogen Bonding and Multiple Metal Binding – A New Cyclic Polyaminopolyalcohol Ligand as Building Block for the Construction of Microporous, Supramolecular Networks

✍ Scribed by Günter J. Merten; Christian Neis; Stefan Stucky; Volker Huch; Eva Rentschler; Harald Natter; Rolf Hempelmann; Klaus Stöwe; Kaspar Hegetschweiler


Publisher
John Wiley and Sons
Year
2011
Tongue
English
Weight
536 KB
Volume
2012
Category
Article
ISSN
1434-1948

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✦ Synopsis


Cyclohexane-based polyaminopolyalcohols (PAPAs) such as 1,3-diamino-1,2,3-trideoxy-cis-inositol (daci) have been prepared by hydrogenation of suitable aromatic precursors. The pentanuclear complex [Cu 5 (daci) 4 (H -2 daci) 2 ](SO 4 ) 3 •18H 2 O (C3) revealed antiferromagnetic and ferromagnetic interactions between the Cu II centers with an S = 3/2 ground state.