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The influence of aromatic cations on the geometries of the Bi(III) halide polyhedra. Synthesis and crystal structures of quinolinium, isoquinolinium and 8-hydroxyquinolinium polychlorobismuthate(III) derivatives

✍ Scribed by Franco Benetollo; Gabriella Bombieri; Antonio Del Pra; Giuseppe Alonzo; Nuccio Bertazzi


Publisher
Elsevier Science
Year
2001
Tongue
English
Weight
270 KB
Volume
319
Category
Article
ISSN
0020-1693

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✦ Synopsis


The compounds [quinolinium] 4 [Bi 2 Cl 10 ] (1), [isoquinolinium]

have been obtained by reacting bismuthate oxide and the appropriate base in HCl acid medium. The crystal structures of 1 and 2 consist of quinolinium and isoquinolinium cations, respectively, interacting through hydrogen bonding with [Bi 2 Cl 10 ] 4 -dimers. The different degree of interactions in the two derivatives causes significant differences in the bond distances of the anions. The crystal structure of 3 is made of [BiCl 6 ] 3 -and Cl -anions and 8-hydroxyquinolinium cations. Hydrogen bond interactions including the N-bonded and O-bonded H atoms together with an interstitial chlorine atom stabilize the entire crystal structure.