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The energetic effects of p, d, and f Gaussian polarization functions on closed-shell AHn oxygen and sulfur hydrides

✍ Scribed by Roy Kari; Imre G. Csizmadia


Publisher
John Wiley and Sons
Year
1977
Tongue
English
Weight
505 KB
Volume
11
Category
Article
ISSN
0020-7608

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✦ Synopsis


Abstract

A series of LCAO‐MO‐SCF calculations, using various basis sets of Gaussian‐type functions, has been made in order to study the effects of p, d, and f polarization functions for a 10‐electron isoelectronic series of oxygen hydrides and for an 18‐electron isoelectronic series of sulfur hydrides. Conclusions from these results suggest that meaningful proton affinities cannot be calculated without the inclusion of a d function on the heavy atom and a p function on the hydrogen atoms.