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The effect of circularly polarized light on ESR spectra

โœ Scribed by A.D. Buckingham; L.C. Parlett

Publisher
Elsevier Science
Year
1995
Tongue
English
Weight
381 KB
Volume
243
Category
Article
ISSN
0009-2614

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โœฆ Synopsis

Observable shifts in electron spin resonance spectra are predicted to occur as a result of the application of circularly polarized light at a frequency near optical absorption. The shift changes sign with the circularity of the light. In a right circularly polarized beam of intensity 10 W cm -2 and frequency 5 GHz above resonance with the D 1 line, propagating in the direction of the magnetic field B z, the electron spin resonance frequency of atomic sodium is predicted to increase by 4.68 MHz. Measurement of the laser-induced shift would determine the antisymmetric polarizability Ollxy = --Ollyx of the radical.

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