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The Cram Rule Revisited Once More — Revision of the Felkin−Anh Model

✍ Scribed by Richard J. Smith; Michael Trzoss; Michael Bühl; Stefan Bienz


Book ID
101350989
Publisher
John Wiley and Sons
Year
2002
Tongue
English
Weight
146 KB
Volume
2002
Category
Article
ISSN
1434-193X

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✦ Synopsis


The reaction mechanism of the LiH addition to α-chiral ketones and acylsilanes was calculated at the ab initio MP2/6-311+G**//RHF/6-31G* level. The selectivities predicted on the basis of the computed transition states and reaction barriers compare well with the experimental data. For compounds possessing very large groups, anti-Cram selectivity