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The challenge of fitting AB initio surfaces. A test of the utility of akima's bivariate interpolation method to dynamical studies

✍ Scribed by S.K. Upadhyay; N. Sathyamurthy


Book ID
103019818
Publisher
Elsevier Science
Year
1982
Tongue
English
Weight
378 KB
Volume
92
Category
Article
ISSN
0009-2614

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✦ Synopsis


The accuracy of a new bivariate method of interpolation in fitting ab initio potential-energy surfaces has been tested by computing coUinear quasiclassical trajectories on the interpolated surface for He + H~ and Li + FH at Eto t = 1.1 and 3.0 eV respectively and comparing the results with those obtained on the original surfaces. It is comparable in reliability and computational time to the spline interpolation procedure.