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tert-Butyldimethylsilyldichloromethyllithium as a dichloromethylene dianion synthon. 1,3-rearrangement of silyl group from carbon to oxide

✍ Scribed by Hiroshi Shinokubo; Katsukiyo Miura; Koichiro Oshima; Kiitiro Utimoto


Publisher
Elsevier Science
Year
1993
Tongue
French
Weight
302 KB
Volume
34
Category
Article
ISSN
0040-4039

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✦ Synopsis


One-pot syatksir of R~H(OS~~~~-~-BII~CC~~CH(OH)R~ by auccurive sdditim of two diffmt damphih haa ban ticvcd startinp from terMmtyldimcthylsiilyldidtl~yRithium. Trcammu 0faTHF sduth d the title cmbanbn with @+4&C,jH4Cm) Or n-BnCHO followed by aa addition of HhiPA and bamddd~ydc &ave the amqmdhg 1.3did monosilyl ether in 83% 0145% yidd. mpectivdy.