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Synthetic studies with [18F]p-fluorobenzenediazonium chloride application to the synthesis of a radiolabelled glucocorticoid: [18F]WIN 44577

✍ Scribed by Anthony L. Feliu


Publisher
John Wiley and Sons
Year
1988
Tongue
French
Weight
405 KB
Volume
25
Category
Article
ISSN
0022-2135

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✦ Synopsis


A route was devised to synthesize no-carrier-added or carrier-added C*uFlp-fluorophenylhydratine from aqueous C'OFlfluoride. Key reaction in this three-step sequence is the reduction o f C1nFlp-fluorobenzenediazonium chloride with sodium cyanoborohydride. The utility of this method is demonstrated by the synthesis of E'FIWIN 44577, an N-(p-fluoropheny1)pyrazole-containing corticosteroid, which exhibits exceptionally high in vitro binding affinity for type-I1 qlucocorticoid receptors, and which is currently under evaluation as a possible radioligand for positron emission tomographic studies.