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Synthetic connections to the aromatic directed metalation reaction. Functionalized aryl boronic acids by ipso borodesilylation. General syntheses of unsymmetrical biphenyls and m-terphenyls

✍ Scribed by M.J. Sharp; W. Cheng; V. Snieckus


Publisher
Elsevier Science
Year
1987
Tongue
French
Weight
272 KB
Volume
28
Category
Article
ISSN
0040-4039

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✦ Synopsis


Aryl boronic acids 2a-d and la-d obtained by metalation-B(OMe)s or metalation silylation-ipso borodesilylation sequences, participate in efficient Pd'-catalyzed cross coupling reactions with aryl bromides to give unsymmetrical biphenyls 3a-d and m_terphenyls 5a-d respectively.

We have recently described1 a general Pd-catalyzed cross coupling protocol2 for the