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Synthetic applications of the tandem aldol condensation-radical cyclization sequence. A new and highly convergent method for the annulation of carbocycles

✍ Scribed by William R. Leonard; Tom Livinghouse


Book ID
104229171
Publisher
Elsevier Science
Year
1985
Tongue
French
Weight
181 KB
Volume
26
Category
Article
ISSN
0040-4039

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✦ Synopsis


The sequential treatment of a,R-unsaturated ketones with (phenylseleno)alanes or -es followed by representative 6,y-unsaturated aldehydes has been shown to furnish B-(phenylseleno)ketols in high yield. The reductive cyclization of these species in the presence of tri-z-butyltin hydride affords the corresponding condensed carbocycles with high efficiency.