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Synthesis and Crystal Structure of a Cocrystalline Compound of a Rare Earth Metalloporphyrin with Fullerene {[TPPYb(μ-OH)2Yb(THF)TPP]·C60}n

✍ Scribed by Jie Zhang; Ruifang Cai; Minqing Chen; Linhong Weng; Xigeng Zhou


Publisher
John Wiley and Sons
Year
2005
Tongue
English
Weight
137 KB
Volume
2005
Category
Article
ISSN
1434-1948

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✦ Synopsis


Abstract

The reaction of YbI~2~(THF)~2~ with TPPLi~2~ (TPP = 5,10,15,20‐tetraphenylporphyrin) in THF, and then with 0.5 equiv. of C~60~, which was solvated in toluene beforehand, gave the title compound {[TPPYb(μ‐OH)~2~Yb(THF)TPP]·C~60~}~n~, which is the first example of a rare earth metallofullerene cocrystal compound. X‐ray structural analyses indicate that this compound displays a complicated supramolecular structure, which contains some unique noncovalent interactionsbetween C~60~ and the rare earth metalloporphyrin units. (© Wiley‐VCH Verlag GmbH & Co. KGaA, 69451 Weinheim, Germany, 2005)