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Synchrotron SAXS and WAXS Studies on Changes in Structural and Thermal Properties of Poly[(R)-3-hydroxybutyrate] Single Crystals during Heating

✍ Scribed by Masahiro Fujita; Tomoharu Sawayanagi; Toshihisa Tanaka; Tadahisa Iwata; Hideki Abe; Yoshiharu Doi; Kazuki Ito; Tetsuro Fujisawa


Publisher
John Wiley and Sons
Year
2005
Tongue
English
Weight
277 KB
Volume
26
Category
Article
ISSN
1022-1336

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✦ Synopsis


Abstract

Summary: The annealing and melting behavior of poly[(R)‐3‐hydroxybutyrate] (P(3HB)) single crystals were followed in real time by synchrotron small‐ (SAXS) and wide‐angle X‐ray scattering (WAXS) measurements. The real‐time SAXS measurements revealed that the P(3HB) single crystal exhibits a discontinuous increase of lamellar thickness during heating. The structural changes as observed by SAXS and WAXS were in response to the thermal properties of single crystals characterized by differential scanning calorimetry.

A series of two‐dimensional small‐angle X‐ray scattering patterns of P(3HB) single crystal mats during the lamellar thickening process.

imageA series of two‐dimensional small‐angle X‐ray scattering patterns of P(3HB) single crystal mats during the lamellar thickening process.