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Swern Oxidation of Alkenyl-Substituted 2-(tert-Butyldimethylsiloxy)-1-(hydroxymethyl)cyclopropanes: A Novel and Flexibel Route to Functionalized 2,5-Dihydrooxepines

✍ Scribed by Hofmann, Bernhard ;Reißig, Hans-Ulrich


Book ID
102776352
Publisher
Wiley (John Wiley & Sons)
Year
1994
Tongue
English
Weight
775 KB
Volume
127
Category
Article
ISSN
0009-2940

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✦ Synopsis


Abstract

Swern oxidation of 2‐alkenyl‐substituted 2‐siloxy‐1‐(hydroxymethyl)cyclopropanes 7 and 11 ‐ 16 provided 2,5‐dihydrooxepines 8 and 17‐21, respectively. The corresponding cyclopropanecarboxaldehydes are highly plausible intermediates in this transformation, which give the seven‐membered heterocycles by a concerted [3,3]‐sigmatropic rearrangement. Some of the 2,5‐dihydrooxepines easily undergo ring contraction to 2‐vinyl‐2,3‐dihydrofurans. Direct formation of these furan derivatives was observed when (hydroxymethyl)‐ cyclopropanes 25‐28 were oxidized. In these cases a step‐wise rearrangement of the 2‐siloxycyclopropanecarboxalde‐hydes involving 1,3‐zwitterions as intermediates is proposed. Our results are compared with the few literature examples and reveal interesting substituent effects. Thus, the donor‐acceptor substitution shifts the equilibrium between the 2‐vinylcyclopropanecarboxaldehydes and the 2,5‐dihydrooxepines to the side of the seven‐membered heterocycles. Further mechanistic details are discussed.