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Surface oxides: carbon containing intermediates at Pt electrodes in relation to the Kolbe reaction

✍ Scribed by E.J. Vasini; M.C. Giordano


Publisher
Elsevier Science
Year
1990
Tongue
English
Weight
651 KB
Volume
35
Category
Article
ISSN
0013-4686

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✦ Synopsis


Potential step techniques and repetitive square wave potential sweeps are applied to Pt electrodes immersed in aqueous acetic-acetate and tritIuoroac&ic-trifluoroacetate solutions to study the initial stages of the Kolbe electrosynthesis reaction and their relation to surface oxides of F't and possible carbon-containing surface intermediates. These results are interpreted through a reaction model in which the Kolbe reaction takes place on a modified R surface involving F't-bonded carbon species.