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Sum-frequency generation from surface species in porous silicon

✍ Scribed by Mattei, G. ;Valentini, V. ;Yakovlev, V. A. ;Mani, A. A. ;Sartenaer, Y. ;Thiry, P. A. ;Peremans, A. ;Caudano, Y. ;Dreesen, L. ;Humbert, C. ;Busson, B. ;Vidal, F. ;Tadjeddine, A.


Publisher
John Wiley and Sons
Year
2005
Tongue
English
Weight
136 KB
Volume
202
Category
Article
ISSN
0031-8965

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✦ Synopsis


Abstract

For the first time, the sum‐frequency generation (SFG) spectra of surface species have been measured in porous silicon (PS) layers. The range of the vibrations 2000–2300 cm^–1^ for the native species Si–H~x~ has been explored. Furthermore for the studied mesoporous materials, it has been found that, as opposed to the infrared absorption, the SFG signal increases with porosity. Finally, the angular dependence and the enhancement of the SFG signal were measured in a one‐dimensional PS photonic crystal structure with a defect producing an energy level in the photonic band gap. (© 2005 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)


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