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Substituent effects on the regioselectivity of enzymatic acylation of 6-O-alkylglycopyranosides using Pseudomonas cepacia lipase

✍ Scribed by David A. MacManus; Evgeny N. Vulfson


Publisher
Elsevier Science
Year
1995
Tongue
English
Weight
730 KB
Volume
279
Category
Article
ISSN
0008-6215

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✦ Synopsis


The regioselectivity of acylation of a range of 6-O-protected glycosides using Pseudomonas cepacia lipase in vinyl acetate was investigated. In general, cY-glycosides were acylated at the O-2 position and P-glycosides were acylated at the O-3 position. The effects of varying the size/hydrophobicity of the O-6 and anomeric substituents on the regioselectivity of the reaction are discussed in terms of the binding of the substrate in the active site of the enzyme.