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Subcellular imaging of isotopically labeled carbon compounds in a biological sample by ion microprobe (NanoSIMS)

✍ Scribed by Peta L. Clode; Richard A. Stern; Alan T. Marshall


Publisher
John Wiley and Sons
Year
2007
Tongue
English
Weight
728 KB
Volume
70
Category
Article
ISSN
1059-910X

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✦ Synopsis


Abstract

Here we demonstrate the technique of nanoscale secondary ion mass spectrometry, utilizing the Cameca NanoSIMS50® ion microprobe, to detect and image the metabolism of an isotopically labeled compound (NaH^13^CO~3~) in a biological sample. In particular, we have designed and verified protocols for imaging the subcellular distribution and determining the relative abundance of labeled ^13^C, within the coral Galaxea fascicularis. Analyses were conducted on 1‐μm thick sections of resin‐embedded material, using both scanned (mapping) and static (spot analysis) Cs^+^ primary ion beam of ∼100 nm diameter. Using these samples we establish that NanoSIMS has adequate mass resolution to reliably distinguish ^13^C from potential isobaric interference by ^12^C^1^H and that data extracted from ion maps are comparable to those acquired by spot analyses. Independent of the method of acquisition, ratioing of ^13^C to the naturally abundant ^12^C is essential if meaningful data, which can be statistically compared to standard and control samples, are to be obtained. These results highlight the potential of NanoSIMS for intracellular tracking of a variety of organic and inorganic compounds labeled with stable isotopes of C, N, O, S, P, and halogens. Microsc. Res. Tech., 2007. © 2007 Wiley‐Liss, Inc.