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Study of the large non-stoichiometry of copper(I) oxide on oxidized copper (T pO2 = 0.21 atm)

✍ Scribed by M. Lenglet; J. M. Machefert; J. M. Claude; B. Lefez; J. Lopitaux; A. D'Huysser


Publisher
John Wiley and Sons
Year
1990
Tongue
English
Weight
321 KB
Volume
16
Category
Article
ISSN
0142-2421

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✦ Synopsis


Abstract

The study of the oxidation of copper at low temperatures shows that the metal is not recovered by a pure stoichiometric Cu~2~O but by a copper(I) oxide phase with the same crystalline structure as Cu~2~O, and that this phase exhibits a very large non‐stoichiometry (composition between Cu~60~O~40~ and Cu~63~O~37~). These results explain that the UV‐Vis‐NIR spectra are different from those of high‐purity Cu~2~O crystals and the position of the absorption bands attributable to defects could be justified easily by the Bohr theory of the hydrogen atom applied to semiconductors.