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Structure-reactivity relationships in triplet sensitized photolysis of aromatic ketone O-acyloximes

✍ Scribed by Hirochika Sakuragi; Masayuki Yoshida; Hideko Kinoshita; Kimie Utena; Katsumi Tokumaru; Masamatsu Hoshino


Book ID
104245648
Publisher
Elsevier Science
Year
1978
Tongue
French
Weight
145 KB
Volume
19
Category
Article
ISSN
0040-4039

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✦ Synopsis


Structure-reactivity relationships in photoreactio;s are of great interest and importance. 1 Previously 0-acyloximes of aromatic ketones were shown to undergo homolytic cleavage at the N-O bond on excitation to their triplet states. 2

We now wish to report on studies designed to determine structural factors responsible for reactivity of the triplet states of aromatic ketone 0-acyloximes.

The mechanism of the triplet sensitized photolysis of the 0-acyloximes is

shown by the following kinetic scheme: