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Structure-reactivity correlation in the reactions of pyrrolidine with O-ethyl S-aryl dithiocarbonates in aqueous ethanol

✍ Scribed by Enrique A. Castro; Mauricio Cabrera; Jose G. Santos


Publisher
John Wiley and Sons
Year
1997
Tongue
English
Weight
64 KB
Volume
29
Category
Article
ISSN
0538-8066

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✦ Synopsis


ethyl S- (2,4,6-trinitrophenyl) dithiocarbonate [1] and a stepwise path through a tetrahedral intermediate in the other reactions [2,3]. In the reaction of O-ethyl Sphenyl dithiocarbonate the zwitterionic tetrahedral intermediate formed by the amine attack can be deprotonated to yield an anionic intermediate in a kinetically significant step [2].

We have also studied the above reactions in water [4] and those of the same amines with the other three Oethyl S-(X-phenyl) dithiocarbonates (X ϭ p-chloro,