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Stereochemical course of the cryptic elimination and cyclization steps in the reaction catalyzed by dehydroquinate synthase

✍ Scribed by Widlanski, Theodore S.; Bender, Steven L.; Knowles, Jeremy R.

Book ID: 126101470
Publisher: American Chemical Society
Year: 1987
Tongue: English
Weight: 415 KB
Volume: 109
Category: Article
ISSN: 0002-7863
DOI: 10.1021/ja00240a054

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## Abstract Application of new chiral ligands (__R__)‐(−)‐**12 a** and (__S__)‐(+)‐**12 c** (VALDY), derived from amino acids, to the title reaction, involving cinnamyl (linear) and isocinnamyl (branched) type substrates (**4** and **5** → **6**), led to excellent regio‐ and enantioselectivities (>