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Stepwise syntheses of unsymmetrical tetra-arylporphyrins. Adaptation of the macdonald dipyrrole self-condensation methodology

✍ Scribed by David M. Wallace; Kevin M. Smith


Book ID
104221858
Publisher
Elsevier Science
Year
1990
Tongue
French
Weight
245 KB
Volume
31
Category
Article
ISSN
0040-4039

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✦ Synopsis


A new synthetic route to meso-tetraarylporphyrins [e.g. (12,13)] using a MacDonald-type 2+2 condensation is established. The method presented here shows wide applicability for the preparation of 5,10,15,20-tetra-arylsubstituted porphyrins with two-fold rotational symmetry. The 2+2 method is further extended to give a tetraqlporphyrin (14) bearing four different aryl groups in a predesignated array.