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Spectroscopy of Σ00→Π10 Vibrational–Tunneling–Rotational Band in Rg · ND3 (Rg = Ne, Ar, Kr)

✍ Scribed by Dmitry G. Melnik; Terry A. Miller; Frank C. De Lucia


Publisher
Elsevier Science
Year
2002
Tongue
English
Weight
241 KB
Volume
214
Category
Article
ISSN
0022-2852

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✦ Synopsis


A number of vibrational-tunneling-rotational (VTR) transitions in the range of 195-298 GHz belonging to the 0 0 → 1 0 hindered rotation band in Rg • ND 3 (Rg = Ne, Kr) complexes are observed in absorption in a free supersonic jet, using the pulsed fast scan submillimeter-wave spectroscopic technique (FASSST). The data obtained in this experiment, combined with previously obtained data on the Ar • ND 3 complex, were used to construct a qualitative model describing the inversion-tunneling motion in the lowest states of the Rg • ND 3 complexes.