## Abstract Recently, the ordinary qualitative criterion on how to distinguish between coherent and incoherent convolutions of broadband coherent anti‐Stokes Raman (CARS) signals generated by degenerate pump lasers has been revised in view of a quantitative analysis. The revision has established th
✦ LIBER ✦
Spectral synthesis of coherent anti-Stokes Raman spectra with broadband Stokes lasers of arbitrary line shapes
✍ Scribed by Michele Marrocco
- Publisher
- John Wiley and Sons
- Year
- 2007
- Tongue
- English
- Weight
- 282 KB
- Volume
- 38
- Category
- Article
- ISSN
- 0377-0486
- DOI
- 10.1002/jrs.1784
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## Abstract Coherent anti‐Stokes Raman scattering (CARS) spectroscopy of gas‐phase CO~2~ is demonstrated using a single femtosecond (fs) laser beam. A shaped ultrashort laser pulse with a transform‐limited temporal width of ∼7 fs and spectral bandwidth of ∼225 nm (∼3500 cm^−1^) is employed for simu