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Some Problems in the Estimation of Chlorophyll-a and Phaeopigments from Pre- and Post-acidification Spectrophotometrie Measurements

✍ Scribed by Dr. Jan R. Moed; Dr. Gustaaf M. Hallegraeff


Publisher
John Wiley and Sons
Year
1978
Tongue
English
Weight
919 KB
Volume
63
Category
Article
ISSN
1434-2944

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✦ Synopsis


The rate of conversion of chlorophyll-a to phaeophytin-a in dilute acid organic solvents is markedly pH-dependent. Tho widely used spectrophotometric measurement before and after acidification to discriminate between chlorophyll-a and phaeopigments is applicnhle only between pH 2.6-2.8. At higher pH the reaction proceeds slowly and occasionally may be incomplete. At lower pH complicating reactions may occur, such as breakdown of certain carotenoid pigments causing (time-dependent) increase of background absorption, and formation of di-cations of phaeophytin with spectral characteristics different from the usually obtained mono-cations of phaeophytin. Consequently, i t is stressed to control carefully the acid concentration, the water content of the solvent, and the amount of MgC03 used in the filtration procedure. I n general, for the purpose of spectrophotometric acidification experiments, acidification by dilute hydrochloric acid added to organic solvents containing 10-200/0 water, and omission of MgCO, would be preferable.

On the basis of observed complications in t h e red p a r t of t h e absorption spectrum of the pigment extract, i t is recommended to use the above stated pH-range.