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Solvation Effects on Geometry and Chemical Shifts. An Ab Initio/IGLO Reconciliation of Apparent Experimental Inconsistencies on H3B · NH3

✍ Scribed by Dipl.-Chem. Michael Bühl; Dr. Thomas Steinke; Prof. Dr. Paul von Ragué Schleyer; Prof. Dr. Roland Boese


Publisher
John Wiley and Sons
Year
1991
Tongue
English
Weight
274 KB
Volume
30
Category
Article
ISSN
0044-8249

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✦ Synopsis


Details of the experimental setup are given elsewhere [lo, 121. A further modification of the high-Dressure cell was undertaken. The samhire win-

dow through which the radiation entered the cell was replaced with a 10 mm thick steel window into which a hole (9 mm deep, 8 mm diameter) was drilled. In this way sufficient radiation for accurate experiments could penetrate the cell. A Xe-Hg arc lamp was used to follow the reaction at 313 nm. the high light intensity of this lamp helped to increase the signalto-noise ratio of the kinetic traces. All experiments were performed at 17°C.

[12] a) R.