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Solid acid porous materials for the catalytic transformation of 1-adamantanol

✍ Scribed by S.P. Elangovan; Katsuki Inoue; Toshiyuki Yokoi; Tatsuya Okubo; Akio Kojima; Masaru Ogura

Publisher: Elsevier Science
Year: 2008
Tongue: English
Weight: 381 KB
Volume: 131
Category: Article
ISSN: 0920-5861
DOI: 10.1016/j.cattod.2007.10.044

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✦ Synopsis

Catalytic transformation of 1-adamantanol has been carried out over nano-porous materials with pore sizes ranging from 0.55 to 6 nm and acidic sites ranging from 0.07 to 4 mmol/g. Zeolites viz., H-USY, H-beta, H-mordenite, H-L and H-ZSM-5, and sulfonic-acid functionalized mesoporous silica viz., MCM-41, SBA-15 and SBA-16, were employed for the reaction. Shape selectivity in a confined micropore plays a role with the combination of medium strength acid sites toward formation of desirable 2-derivatives, which comprises a maximum amount of 2adamantanone.

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