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Singlet Oxygen and the Production of Sulfur Oxygenates of Nickel(II) and Palladium(II) Thiolates

✍ Scribed by Grapperhaus, Craig A.; Maguire, Michael J.; Tuntulani, Thawatchai; Darensbourg, Marcetta Y.

Book ID: 127386121
Publisher: American Chemical Society
Year: 1997
Tongue: English
Weight: 335 KB
Volume: 36
Category: Article
ISSN: 0020-1669
DOI: 10.1021/ic970050d

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## Abstract In the Ni(II)–S(IV)–O~2~ system in the region of pH > 8.4, both Ni(II) and S(IV) are simultaneously autoxidized, and when sulfur is consumed fully NiOOH precipitates. At pH > 8.4, ethanol has no effect on the rate, whereas ammonia strongly inhibits the reaction when pH > 7.0. The kineti