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Simultaneous intraparticle forced convection, diffusion and reaction in a porous catalyst

✍ Scribed by Nir Avinoam; Pismen Leonid M


Publisher
Elsevier Science
Year
1977
Tongue
English
Weight
602 KB
Volume
32
Category
Article
ISSN
0009-2509

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✦ Synopsis


Ah&act-The effect of mtrapmcle forced convection on a heterogeneous reaction wlthm a porous cat&W pellet IS exammed It IS found that an appreciable enhancement of the catalyst performance can be. expected for hqmd-phase reactions on coarse-gzamed pmcles Quantitatwe results are obtamed for an ureverslble Isothermal &t-order reaction UI flat, spherical and cylmdr~cal geometries with umform Internal flow A maxunum mcrease m the effectiveness factor 1s observed in the reDon where the hnetics Just becomes dtiuslon controlled


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Ah&r&-The effect of intraparticle forced convection on the effectiveness of a porous catalyst was studied experimentally. Depolymerization of paraldehyde, catalysed by nickel-sulfate supported on cylindrical pellet of porous silica-gel, was measured in a basket-type reactor. The effective reaction r

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## Abstract Intraparticle forced convection was considered in order to explain experimentally observed changes in effective diffusivity (apparent) with flowrate, when measures are carried out in fixed beds. A complete model taking into account intraparticle diffusion and forced convection together

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## Abstract The problem of simultaneous convection, diffusion and reaction inside a porous catalyst slab is considered. A combination of perturbation and integral mathematical techniques are used to derive approximate analytical solutions for the concentration and temperature profiles, as well as f