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Simultaneous determination by UPLC–ESI-MS of scoparone, capillarisin, rhein, and emodin in rat urine after oral administration of Yin Chen Hao Tang preparation

✍ Scribed by Haitao Lv; Hui Sun; Xijun Wang; Wenjun Sun; Guozheng Jiao; Dixin Zhou; Li Zhao; Hongxin Cao; Guangmei Zhang


Publisher
John Wiley and Sons
Year
2008
Tongue
English
Weight
936 KB
Volume
31
Category
Article
ISSN
1615-9306

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✦ Synopsis


Abstract

A simple, sensitive, and validated method was developed for simultaneous determination of scoparone, capillarisin, rhein, and emodin in rat urine by ultra‐performance liquid chromatography/electrospray ionization quadruple time‐of‐flight mass spectrometry (UPLC–MS). The urinary samples were analyzed on an Acquity UPLC BEH C~18~ 1.7 μm 2.1×50 mm column. Scoparone, capillarisin, rhein, and emodin in rat urine were simultaneously analyzed with good separation. The lower limits of detection were 6.0, 9.0, 7.0, and 3.0 ng/mL, and the lower limits of quantification were 20.0, 33.0, 24.0, and 12.0 ng/mL for scoparone, capillarisin, rhein, and emodin, respectively. The intra‐ and inter‐day precisions (RSD) were less than 9%. The intra‐ and inter‐accuracies were found to be in the range of 94.14–104.54% for scoparone, 101.72–107.34% for capillarisin, 95.24–103.59% for rhein, and 101.32–107.82% for emodin at three concentration levels. The absolute recoveries for scoparone, capillarisin, rhein, and emodin were not less than 77.0%. The developed method has been applied to determine scoparone, capillarisin, rhein, and emodin in rat urine after oral administration of Yin Chen Hao Tang preparation, a traditional Chinese medicine formulation widely used in China for treatment of jaundice and liver disorders.