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Selected fluorescence and dissociation lifetimes on N2O+ in its Ã(2Σ+),000 and 100 states

✍ Scribed by R. Frey; B. Gotchev; W.B. Peatman; H. Pollak; E.W. Schlag

Publisher: Elsevier Science
Year: 1978
Tongue: English
Weight: 299 KB
Volume: 54
Category: Article
ISSN: 0009-2614
DOI: 10.1016/0009-2614(78)85250-6

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✦ Synopsis

Radiative and radiationless lifetimes together with the quantum yield towards fluorescence of mdividual vlbrontc states of molecular IOIIS can be determined by threshold electron-fluorescence photon coincidence measurements. This method is here applied to the % %I~/~ I,t and x *2+ states of N20* which were also studied by high resolutlon photoionizatlon reso-, nance spectroscopy.

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The reaction C( 'P) +NsO(% \*C+) is studied by varying the kinetic energy of C(3P) in two center-of-mass regimes: 0.1-0.2 eV and 2-7 eV. C( 3P) is directly observed, and the C, velocity distribution is estimated from the time-of-flight of Cs. CN(X %+) is vibrationally inverted and rotationally 'hot'