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Ruthenium-Catalyzed Cascade N- and C(3)-Dialkylation of Cyclic Amines with Alcohols Involving Hydrogen Autotransfer Processes

✍ Scribed by Basker Sundararaju; Zhou Tang; Mathieu Achard; Gangavaram V. M. Sharma; Loïc Toupet; Christian Bruneau

Publisher
John Wiley and Sons
Year
2010
Tongue
English
Weight
266 KB
Volume
352
Category
Article
ISSN
1615-4150

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✦ Synopsis

Abstract

An unprecented N‐ and C(3)‐dialkylation of unactivated amines by a cascade reaction via borrowing hydrogen methodology using new (arene)ruthenium(II) complexes featuring phosphinosulfonate ligands is described. This reaction is highly regioselective and produces water as the only side product.

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