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Rotational barriers of disilane, hexafluorodisilane, and hexamethyldisilane:Ab initio, density functional, and molecular mechanics (MM3) studies

✍ Scribed by Cho, Soo Gyeong; Rim, One Kwon; Park, Gyoosoon


Publisher
John Wiley and Sons
Year
1997
Tongue
English
Weight
169 KB
Volume
18
Category
Article
ISSN
0192-8651

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✦ Synopsis


‡ Ž . ⌬G 298 K values were in good agreement with experimental values published recently. In addition, we also performed MM3 calculations on Si H and 2 6 Si Me . MM3 calculated rotational barriers and thermodynamic properties were 2 6 compared with high level ab initio results. Based on this comparison, MM3 calculations reproduced high level ab initio results in rotational barriers and thermodynamic properties of Si H derivatives including vibrational energies 2 6

and entropies, although large errors exist in some vibrational frequencies.