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Rhodium-Catalyzed Direct Oxidative Carbonylation of Aromatic C−H Bond with CO and Alcohols

✍ Scribed by Guan, Zheng-Hui; Ren, Zhi-Hui; Spinella, Stephen M.; Yu, Shichao; Liang, Yong-Min; Zhang, Xumu

Book ID
120814117
Publisher
American Chemical Society
Year
2009
Tongue
English
Weight
161 KB
Volume
131
Category
Article
ISSN
0002-7863

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The reaction of N-acylpiperazineswith CO (15 arm) and ethylene at 160 'C in the presenceof Rh4(CO),2results in dehydrogenation and carbonylationat a C-H bond. This ceaction representsthe first exampleof carbonylationat a C-H bondpromotedby an oxygenfunctionalgroup.