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Reversed-phase liquid chromatography of the twenty-two tetrachlorodibenzo-p-dioxin isomers on pyrenylethyl- and octadecylsilylated silica gel columns

✍ Scribed by Elizabeth R. Barnhart; Donald G. Patterson Jr.; Nobuo Tanaka; Mikio Araki


Book ID
104145725
Publisher
Elsevier Science
Year
1988
Tongue
English
Weight
698 KB
Volume
445
Category
Article
ISSN
1873-3778

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✦ Synopsis


To purify the tetrachlorobenzo-p-dioxins synthesized for chemical and biological reference standards, reversed-phase liquid chromatography on pyrenylethyl-and octadecylsilylated stationary phase (PYE and Crs) columns was employed with 100% methanol. The pyrenylethyl phase satisfactorily separated isomers resulting from mixtures of reaction products which had not been adequately separated with conventional Cis or silica gel. The use of a single chromatographic mode, liquid chromatography, and a single mobile phase with columns of distinctly different properties, Cle and PYE, separates 20 of the 22 isomers from each other and from the 1246/1249 pair. (The observed properties of the two columns afford insight into steric and polarizability differences among isomers.) l Use of trade names is for identification only and does not constitute endorsement by the Public Health Service or the U.S. Deuartment of Health and Human Services.