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Relationship between conformation and geometry as evidenced by molecular dynamics simulation of Cα,α-dialkylated glycines

✍ Scribed by Maurizio Cirilli; Vincenza Maria Coiro; Alfredo Di Nola; Fernando Mazza


Publisher
Wiley (John Wiley & Sons)
Year
1998
Tongue
English
Weight
104 KB
Volume
46
Category
Article
ISSN
0006-3525

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✦ Synopsis


The relationship between the local backbone conformation and bond angles at C a of symmetrically substituted C a,a -dialkylated glycines (C a,a -dimethylglycine or a-aminoisobutyric acid, Aib; C a,a -diethylglycine, Deg; C a,a -di-n-propylglycine, Dpg) has been investigated by molecular dynamics (MD) simulation adopting flat bottom harmonic potentials, instead of the usual harmonic restraints, for the C a bond angles. The MD simulations show that the C a bond angles are related to the local backbone conformation, irrespectively of the side-chain length of Aib, Deg, and Dpg residues. Moreover, the N-C a -C (t) angle is the most sensitive conformational parameter and, in the folded form, is always larger and more flexible than in the extended one.