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Relation between Structure and Proton Donor Strength of Octahedrally Coordinated Tris(3,5-diisopropylsalicylato)-aluminum(III), -gallium(III), and -indium(III)

✍ Scribed by Dr. H. F. Eicke; V. Arnold; Dr. F. L'Eplattenier


Publisher
John Wiley and Sons
Year
1972
Tongue
English
Weight
210 KB
Volume
11
Category
Article
ISSN
0044-8249

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✦ Synopsis


from partially fluorinated compounds by distillation at 12 torr. [(NSOCI),(NSOF)] and [(NSOCI)(NSOF),] are isolated by further distillation in a spinning band column. The cis-trans isomers of [NSOF], were separated gaschromatographically and their physical properties were determined. These were in complete agreement with those reported in the literature13! The colorless compounds [(NSOCI), (NSOF)], b. p. 105 to l10°C/20 torr, and [(NSOCI)(NSOF),], b. p. 168 to 175 "C/760 torr, each occur in three isomeric forms, which are completely separable by analytical gaschromatography and which can be characterized by the 19F-NMR spectrum. Trioxodichlorofluorocyclotrithiazene [(NSOCl),(N SOF)] : Mass spectrum (rel. intensity in %): N 3 S 3 0 3 F C l ~ (I), N3S,0,FCI+ (7), N,S,O,F+ (21), NS,OZ (I), NSOCl+ (2). SOCl' (37), SOF' (IOO), NSO' (9), SO+ (43). IR [cm-'1: 1350 (vs), 1205 (w), 1133 (vs), 837 (s), 768 (vs), cis -cis P * CIS-trans Relation between Structure and Proton Donor Strength of Octahedrally Coordinated Tris(3,5-di-isopropylsalicy1ato)-aluminum( HI), -gallium( III), and -indium(m)