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Regiospecific friedel-crafts acylationof 6-alkoxy-2-pyrones: Preparation of substituted aromatics and anthraquinones.

✍ Scribed by Michael E. Jung; Richard W. Brown


Book ID
104234235
Publisher
Elsevier Science
Year
1981
Tongue
French
Weight
265 KB
Volume
22
Category
Article
ISSN
0040-4039

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✦ Synopsis


Friedel-Crafts acylation of 6-alkoxy-2-pyrones gives high yields of the 5-acyl-2-pyrones which undergo regioselective cycloaddition with various dienophiles. Adriamycin 1 and daunorubicin 1. are the anthracycline antitumor agents used most extensively in cancer chemotherapy today.2 Their use is limited by their severe cumulative cardiotoxicity.2 Several 11-desoxyanthracyclines have been isolated in the last few years, e.g., aclacinomycin 3 and 11-desoxy. adriamycin 4, which exhibit good antitumor properties and, more importantly, show lower cardiotoxicity.d c$gYs Recently, we reported the results of a facile preparation of tricyclic analogues