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Regioselective pyrrole synthesis from asymmetric β-diketone and conversion to sterically hindered porphyrin

✍ Scribed by Hiroshi Fujii; Tetsuhiko Yoshimura; Hitoshi Kamada


Book ID
104256412
Publisher
Elsevier Science
Year
1997
Tongue
French
Weight
208 KB
Volume
38
Category
Article
ISSN
0040-4039

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✦ Synopsis


The condensation of asymmetric I~-diketones with (x-oximinoacetoacetate esters affords pyrroles regioselectively. The mechanism of the regioselectivity is studied using ~C-NMR spectroscopy. Pyrrole having a neopentyl group at the 4-position is synthesized by the method, and further converted to a steric hindered porphyrin in good yield.