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Reaktion an Ziegler-Natta-Katalysatoren, 15. Einführung von halogenierten Aralkyl-Gruppen in 1,4-polybutadien und metathese-abbau der modifizierten polymeren

✍ Scribed by Demel, Hans ;Hummel, Klaus


Publisher
Wiley (John Wiley & Sons)
Year
1977
Weight
325 KB
Volume
178
Category
Article
ISSN
0025-116X

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✦ Synopsis


Abstract

1,4‐Polybutadiene was partially aralkylated with halogenated alkylbenzenes (4‐fluorotoluene, 2‐, 3‐, and 4‐chlorotoluene, 4‐bromotoluene, 2‐chloro‐p‐xylene, 2,4‐dichlorotoluene, 3,4‐dichlorotoluene) and dicumyl peroxide. The modified polymers were investigated by IR‐spectroscopy and degraded by olefin metathesis reaction with 4‐octene. The degradation products were separated by gas chromatography and identified by mass spectrometry. In addition to the aralkylation methylation of the 1,4‐polybutadiene occurred.